diff --git a/mlir/include/mlir/Dialect/LLVMIR/LLVMOps.td b/mlir/include/mlir/Dialect/LLVMIR/LLVMOps.td
--- a/mlir/include/mlir/Dialect/LLVMIR/LLVMOps.td
+++ b/mlir/include/mlir/Dialect/LLVMIR/LLVMOps.td
@@ -1648,7 +1648,8 @@
     OptionalAttr<UnitAttr>:$arm_streaming,
     OptionalAttr<UnitAttr>:$arm_locally_streaming,
     OptionalAttr<StrAttr>:$section,
-    OptionalAttr<UnnamedAddr>:$unnamed_addr
+    OptionalAttr<UnnamedAddr>:$unnamed_addr,
+    OptionalAttr<I64Attr>:$alignment
   );
 
   let regions = (region AnyRegion:$body);
diff --git a/mlir/lib/Target/LLVMIR/ModuleImport.cpp b/mlir/lib/Target/LLVMIR/ModuleImport.cpp
--- a/mlir/lib/Target/LLVMIR/ModuleImport.cpp
+++ b/mlir/lib/Target/LLVMIR/ModuleImport.cpp
@@ -1749,6 +1749,9 @@
   if (func->hasComdat())
     funcOp.setComdatAttr(comdatMapping.lookup(func->getComdat()));
 
+  if (llvm::MaybeAlign maybeAlign = func->getAlign())
+    funcOp.setAlignment(maybeAlign->value());
+
   // Handle Function attributes.
   processFunctionAttributes(func, funcOp);
 
diff --git a/mlir/lib/Target/LLVMIR/ModuleTranslation.cpp b/mlir/lib/Target/LLVMIR/ModuleTranslation.cpp
--- a/mlir/lib/Target/LLVMIR/ModuleTranslation.cpp
+++ b/mlir/lib/Target/LLVMIR/ModuleTranslation.cpp
@@ -1044,6 +1044,9 @@
 
     if (auto unnamedAddr = function.getUnnamedAddr())
       llvmFunc->setUnnamedAddr(convertUnnamedAddrToLLVM(*unnamedAddr));
+
+    if (auto alignment = function.getAlignment())
+      llvmFunc->setAlignment(llvm::MaybeAlign(*alignment));
   }
 
   return success();
diff --git a/mlir/test/Dialect/LLVMIR/func.mlir b/mlir/test/Dialect/LLVMIR/func.mlir
--- a/mlir/test/Dialect/LLVMIR/func.mlir
+++ b/mlir/test/Dialect/LLVMIR/func.mlir
@@ -207,7 +207,13 @@
 
   // CHECK-LABEL: local_unnamed_addr @local_unnamed_addr_func
   llvm.func local_unnamed_addr @local_unnamed_addr_func() {
-      llvm.return
+    llvm.return
+  }
+
+  // CHECK-LABEL: @align_func
+  // CHECK-SAME: attributes {alignment = 2 : i64}
+  llvm.func @align_func() attributes {alignment = 2 : i64} {
+    llvm.return
   }
 
   // CHECK: llvm.comdat @__llvm_comdat
diff --git a/mlir/test/Target/LLVMIR/Import/function-attributes.ll b/mlir/test/Target/LLVMIR/Import/function-attributes.ll
--- a/mlir/test/Target/LLVMIR/Import/function-attributes.ll
+++ b/mlir/test/Target/LLVMIR/Import/function-attributes.ll
@@ -229,3 +229,17 @@
 
 ; CHECK-LABEL: unnamed_addr @unnamed_addr_func
 declare void @unnamed_addr_func() unnamed_addr
+
+// -----
+
+; CHECK-LABEL: @align_func
+; CHECK-SAME: attributes {alignment = 2 : i64}
+define void @align_func() align 2 {
+  ret void
+}
+
+// -----
+
+; CHECK-LABEL: @align_decl
+; CHECK-SAME: attributes {alignment = 64 : i64}
+declare void @align_decl() align 64
diff --git a/mlir/test/Target/LLVMIR/llvmir.mlir b/mlir/test/Target/LLVMIR/llvmir.mlir
--- a/mlir/test/Target/LLVMIR/llvmir.mlir
+++ b/mlir/test/Target/LLVMIR/llvmir.mlir
@@ -1656,6 +1656,20 @@
 
 // -----
 
+// CHECK-LABEL: @align_func
+// CHECK-SAME: align 2
+llvm.func @align_func() attributes {alignment = 2 : i64} {
+    llvm.return
+}
+
+// -----
+
+// CHECK-LABEL: @align_decl
+// CHECK-SAME: align 64
+llvm.func @align_decl() attributes {alignment = 64 : i64}
+
+// -----
+
 // CHECK-LABEL: @callFreezeOp
 llvm.func @callFreezeOp(%x : i32) {
   // CHECK: freeze i32 %{{[0-9]+}}